NSData *dataObject = [aString dataUsingEncoding:NSUnicodeStringEncoding];
(or substitute any of the list below for "NSUnicodeStringEncoding" depending on the encoding of your string)
Is this what you've tried?
Other encoding types (from the documentation)
enum {
NSASCIIStringEncoding = 1,
NSNEXTSTEPStringEncoding = 2,
NSJapaneseEUCStringEncoding = 3,
NSUTF8StringEncoding = 4,
NSISOLatin1StringEncoding = 5,
NSSymbolStringEncoding = 6,
NSNonLossyASCIIStringEncoding = 7,
NSShiftJISStringEncoding = 8,
NSISOLatin2StringEncoding = 9,
NSUnicodeStringEncoding = 10,
NSWindowsCP1251StringEncoding = 11,
NSWindowsCP1252StringEncoding = 12,
NSWindowsCP1253StringEncoding = 13,
NSWindowsCP1254StringEncoding = 14,
NSWindowsCP1250StringEncoding = 15,
NSISO2022JPStringEncoding = 21,
NSMacOSRomanStringEncoding = 30,
NSProprietaryStringEncoding = 65536
};